125 research outputs found
Harnessing nuclear spin polarization fluctuations in a semiconductor nanowire
Soon after the first measurements of nuclear magnetic resonance (NMR) in a
condensed matter system, Bloch predicted the presence of statistical
fluctuations proportional to in the polarization of an ensemble of
spins. First observed by Sleator et al., so-called "spin noise" has
recently emerged as a critical ingredient in nanometer-scale magnetic resonance
imaging (nanoMRI). This prominence is a direct result of MRI resolution
improving to better than 100 nm^3, a size-scale in which statistical spin
fluctuations begin to dominate the polarization dynamics. We demonstrate a
technique that creates spin order in nanometer-scale ensembles of nuclear spins
by harnessing these fluctuations to produce polarizations both larger and
narrower than the natural thermal distribution. We focus on ensembles
containing ~10^6 phosphorus and hydrogen spins associated with single InP and
GaP nanowires (NWs) and their hydrogen-containing adsorbate layers. We monitor,
control, and capture fluctuations in the ensemble's spin polarization in
real-time and store them for extended periods. This selective capture of large
polarization fluctuations may provide a route for enhancing the weak magnetic
signals produced by nanometer-scale volumes of nuclear spins. The scheme may
also prove useful for initializing the nuclear hyperfine field of electron spin
qubits in the solid-state.Comment: 18 pages, 5 figure
Nuclear Magnetic Resonance Imaging with 90 nm Resolution
Magnetic resonance imaging, based on the manipulation and detection of
nuclear spins, is a powerful imaging technique that typically operates on the
scale of millimeters to microns. Using magnetic resonance force microscopy, we
have demonstrated that magnetic resonance imaging of nuclear spins can be
extended to a spatial resolution better than 100 nm. The two-dimensional
imaging of 19F nuclei was done on a patterned CaF2 test object, and was enabled
by a detection sensitivity of roughly 1200 nuclear spins. To achieve this
sensitivity, we developed high-moment magnetic tips that produced field
gradients up to 1.4x10^6 T/m, and implemented a measurement protocol based on
force-gradient detection of naturally occurring spin fluctuations. The
resulting detection volume of less than 650 zl represents 60,000x smaller
volume than previous NMR microscopy and demonstrates the feasibility of pushing
magnetic resonance imaging into the nanoscale regime.Comment: 24 pages, 5 figure
An off-board quantum point contact as a sensitive detector of cantilever motion
Recent advances in the fabrication of microelectromechanical systems (MEMS)
and their evolution into nanoelectromechanical systems (NEMS) have allowed
researchers to measure extremely small forces, masses, and displacements. In
particular, researchers have developed position transducers with resolution
approaching the uncertainty limit set by quantum mechanics. The achievement of
such resolution has implications not only for the detection of quantum behavior
in mechanical systems, but also for a variety of other precision experiments
including the bounding of deviations from Newtonian gravity at short distances
and the measurement of single spins. Here we demonstrate the use of a quantum
point contact (QPC) as a sensitive displacement detector capable of sensing the
low-temperature thermal motion of a nearby micromechanical cantilever.
Advantages of this approach include versatility due to its off-board design,
compatibility with nanoscale oscillators, and, with further development, the
potential to achieve quantum limited displacement detection.Comment: 5 pages, 5 figure
Magnetic Resonance Force Microscopy of paramagnetic electron spins at millikelvin temperatures
Magnetic Resonance Force Microscopy (MRFM) is a powerful technique to detect
a small number of spins that relies on force-detection by an ultrasoft
magnetically tipped cantilever and selective magnetic resonance manipulation of
the spins. MRFM would greatly benefit from ultralow temperature operation,
because of lower thermomechanical noise and increased thermal spin
polarization. Here, we demonstrate MRFM operation at temperatures as low as 30
mK, thanks to a recently developed SQUID-based cantilever detection technique
which avoids cantilever overheating. In our experiment, we detect dangling bond
paramagnetic centers on a silicon surface down to millikelvin temperatures.
Fluctuations of such kind of defects are supposedly linked to 1/f magnetic
noise and decoherence in SQUIDs as well as in several superconducting and
single spin qubits. We find evidence that spin diffusion plays a key role in
the low temperature spin dynamics.Comment: 7 pages, 5 figure
Dynamical Axion Field in Topological Magnetic Insulators
Axions are very light, very weakly interacting particles postulated more than
30 years ago in the context of the Standard Model of particle physics. Their
existence could explain the missing dark matter of the universe. However,
despite intensive searches, they have yet to be detected. In this work, we show
that magnetic fluctuations of topological insulators couple to the
electromagnetic fields exactly like the axions, and propose several experiments
to detect this dynamical axion field. In particular, we show that the axion
coupling enables a nonlinear modulation of the electromagnetic field, leading
to attenuated total reflection. We propose a novel optical modulators device
based on this principle.Comment: 5 pages, 3 figure
High-sensitivity diamond magnetometer with nanoscale resolution
We present a novel approach to the detection of weak magnetic fields that
takes advantage of recently developed techniques for the coherent control of
solid-state electron spin quantum bits. Specifically, we investigate a magnetic
sensor based on Nitrogen-Vacancy centers in room-temperature diamond. We
discuss two important applications of this technique: a nanoscale magnetometer
that could potentially detect precession of single nuclear spins and an optical
magnetic field imager combining spatial resolution ranging from micrometers to
millimeters with a sensitivity approaching few femtotesla/Hz.Comment: 29 pages, 4 figure
Ultrasensitive force and displacement detection using trapped ions
The ability to detect extremely small forces is vital for a variety of
disciplines including precision spin-resonance imaging, microscopy, and tests
of fundamental physical phenomena. Current force-detection sensitivity limits
have surpassed 1 (atto ) through coupling of micro or
nanofabricated mechanical resonators to a variety of physical systems including
single-electron transistors, superconducting microwave cavities, and individual
spins. These experiments have allowed for probing studies of a variety of
phenomena, but sensitivity requirements are ever-increasing as new regimes of
physical interactions are considered. Here we show that trapped atomic ions are
exquisitely sensitive force detectors, with a measured sensitivity more than
three orders of magnitude better than existing reports. We demonstrate
detection of forces as small as 174 (yocto ), with a
sensitivity 390 using crystals of Be
ions in a Penning trap. Our technique is based on the excitation of normal
motional modes in an ion trap by externally applied electric fields, detection
via and phase-coherent Doppler velocimetry, which allows for the discrimination
of ion motion with amplitudes on the scale of nanometers. These experimental
results and extracted force-detection sensitivities in the single-ion limit
validate proposals suggesting that trapped atomic ions are capable of detecting
of forces with sensitivity approaching 1 . We anticipate that
this demonstration will be strongly motivational for the development of a new
class of deployable trapped-ion-based sensors, and will permit scientists to
access new regimes in materials science.Comment: Expanded introduction and analysis. Methods section added. Subject to
press embarg
Nonlinear damping in mechanical resonators based on graphene and carbon nanotubes
Carbon nanotubes and graphene allow fabricating outstanding nanomechanical
resonators. They hold promise for various scientific and technological
applications, including sensing of mass, force, and charge, as well as the
study of quantum phenomena at the mesoscopic scale. Here, we have discovered
that the dynamics of nanotube and graphene resonators is in fact highly exotic.
We propose an unprecedented scenario where mechanical dissipation is entirely
determined by nonlinear damping. As a striking consequence, the quality factor
Q strongly depends on the amplitude of the motion. This scenario is radically
different from that of other resonators, whose dissipation is dominated by a
linear damping term. We believe that the difference stems from the reduced
dimensionality of carbon nanotubes and graphene. Besides, we exploit the
nonlinear nature of the damping to improve the figure of merit of
nanotube/graphene resonators.Comment: main text with 4 figures, supplementary informatio
Quantum control of proximal spins using nanoscale magnetic resonance imaging
Quantum control of individual spins in condensed matter systems is an
emerging field with wide-ranging applications in spintronics, quantum
computation, and sensitive magnetometry. Recent experiments have demonstrated
the ability to address and manipulate single electron spins through either
optical or electrical techniques. However, it is a challenge to extend
individual spin control to nanoscale multi-electron systems, as individual
spins are often irresolvable with existing methods. Here we demonstrate that
coherent individual spin control can be achieved with few-nm resolution for
proximal electron spins by performing single-spin magnetic resonance imaging
(MRI), which is realized via a scanning magnetic field gradient that is both
strong enough to achieve nanometric spatial resolution and sufficiently stable
for coherent spin manipulations. We apply this scanning field-gradient MRI
technique to electronic spins in nitrogen-vacancy (NV) centers in diamond and
achieve nanometric resolution in imaging, characterization, and manipulation of
individual spins. For NV centers, our results in individual spin control
demonstrate an improvement of nearly two orders of magnitude in spatial
resolution compared to conventional optical diffraction-limited techniques.
This scanning-field-gradient microscope enables a wide range of applications
including materials characterization, spin entanglement, and nanoscale
magnetometry.Comment: 7 pages, 4 figure
Ultrasensitive force detection with a nanotube mechanical resonator
Since the advent of atomic force microscopy, mechanical resonators have been
used to study a wide variety of phenomena, such as the dynamics of individual
electron spins, persistent currents in normal metal rings, and the Casimir
force. Key to these experiments is the ability to measure weak forces. Here, we
report on force sensing experiments with a sensitivity of 12 zN Hz^(-1/2) at a
temperature of 1.2 K using a resonator made of a carbon nanotube. An
ultra-sensitive method based on cross-correlated electrical noise measurements,
in combination with parametric downconversion, is used to detect the
low-amplitude vibrations of the nanotube induced by weak forces. The force
sensitivity is quantified by applying a known capacitive force. This detection
method also allows us to measure the Brownian vibrations of the nanotube down
to cryogenic temperatures. Force sensing with nanotube resonators offers new
opportunities for detecting and manipulating individual nuclear spins as well
as for magnetometry measurements.Comment: Early version. To be published in Nature Nanotechnolog
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